Department of Chemistry

portrait of Professor John Pyle FRS

Professor John Pyle FRS

St Catharine's College

Groups: Atmospheric group website

Telephone: 01223 336473

E-mail: john.pyle@atm.ch.cam.ac.uk

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling. The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling. We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements. We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Multimodel assessment of the upper troposphere and lower stratosphere: Extratropics
MI Hegglin, A Gettelman, P Hoor, R Krichevsky, GL Manney, LL Pan, SW Son, G Stiller, S Tilmes, KA Walker, V Eyring, TG Shepherd, D Waugh, H Akiyoshi, JA Anel, J Austin, A Baumgaertner, S Bekki, P Braesicke, C Bruhl, N Butchart, M Chipperfield, M Dameris, S Dhomse, S Frith, H Garny, SC Hardiman, P Jockel, DE Kinnison, JF Lamarque, E Mancini, M Michou, O Morgenstern, T Nakamura, D Olivie, S Pawson, G Pitari, DA Plummer, JA Pyle, E Rozanov, JF Scinocca, K Shibata, D Smale, H Teyssedre, W Tian, Y Yamashita - Journal of Geophysical Research D: Atmospheres (2010) 115, ARTN D00M09
(DOI: 10.1029/2010JD013884)
Impact of stratospheric ozone on Southern Hemisphere circulation change: A multimodel assessment
SW Son, EP Gerber, J Perlwitz, LM Polvani, NP Gillett, KH Seo, V Eyring, TG Shepherd, D Waugh, H Akiyoshi, J Austin, A Baumgaertner, S Bekki, P Braesicke, C Bruhl, N Butchart, MP Chipperfield, D Cugnet, M Dameris, S Dhomse, S Frith, H Garny, R Garcia, SC Hardiman, P Jockel, JF Lamarque, E Mancini, M Marchand, M Michou, T Nakamura, O Morgenstern, G Pitari, DA Plummer, J Pyle, E Rozanov, JF Scinocca, K Shibata, D Smale, H Teyssedre, W Tian, Y Yamashita - Journal of Geophysical Research D: Atmospheres (2010) 115, D00M07
(DOI: 10.1029/2010JD014271)
Stratosphere-troposphere coupling and annular mode variability in chemistry-climate models
EP Gerber, MP Baldwin, H Akiyoshi, J Austin, S Bekki, P Braesicke, N Butchart, M Chipperfield, M Dameris, S Dhomse, SM Frith, RR Garcia, H Garny, A Gettelman, SC Hardiman, A Karpechko, M Marchand, O Morgenstern, JE Nielsen, S Pawson, T Peter, DA Plummer, JA Pyle, E Rozanov, JF Scinocca, TG Shepherd, D Smale - Journal of Geophysical Research D: Atmospheres (2010) 115, D00M06
(DOI: 10.1029/2009JD013770)
Anthropogenic forcing of the Northern Annular Mode in CCMVal-2 models
O Morgenstern, H Akiyoshi, S Bekki, P Braesicke, N Butchart, MP Chipperfield, D Cugnet, M Deushi, SS Dhomse, RR Garcia, A Gettelman, NP Gillett, SC Hardiman, J Jumelet, DE Kinnison, JF Lamarque, F Lott, M Marchand, M Michou, T Nakamura, D Olivie, T Peter, D Plummer, JA Pyle, E Rozanov, D Saint-Martin, JF Scinocca, K Shibata, M Sigmond, D Smale, H Teyssedre, W Tian, A Voldoire, Y Yamashita - Journal of Geophysical Research D: Atmospheres (2010) 115, D00M03
(DOI: 10.1029/2009JD013347)
Impact of stratospheric ozone recovery on tropospheric ozone and its budget
G Zeng, O Morgenstern, P Braesicke, JA Pyle - Geophysical Research Letters (2010) 37, ARTN L09805
(DOI: 10.1029/2010GL042812)
Global chemistry simulations in the amma multimodel intercomparison project
JE Williams, R Scheele, P van Velthoven, I Bouarar, K Law, B Josse, VH Peuch, X Yang, J Pyle, V Thouret, B Barret, C Liousse, F Hourdin, S Szopa, A Cozic - Bulletin of the American Meteorological Society (2010) 91, 611
(DOI: 10.1175/2009BAMS2818.1)
Assessment of the breakup of the Antarctic polar vortex in two new chemistry-climate models
MM Hurwitz, PA Newman, F Li, LD Oman, O Morgenstern, P Braesicke, JA Pyle - JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (2010) 115, ARTN D07105
(DOI: 10.1029/2009JD012788)
Tropical deep convection and its impact on composition in global and mesoscale models-part 2: Tracer transport
CR Hoyle, V Marécal, MR Russo, J Arteta, C Chemel, MP Chipperfield, F D'Amato, O Dessens, W Feng, NRP Harris, JS Hosking, O Morgenstern, T Peter, JA Pyle, T Reddmann, NAD Richards, PJ Telford, W Tian, S Viciani, O Wild, X Yang, G Zeng - Atmospheric Chemistry and Physics Discussions (2010) 10, 20355
The potential to narrow uncertainty in projections of stratospheric ozone over the 21st century
AJ Charlton-Perez, E Hawkins, V Eyring, I Cionni, GE Bodeker, DE Kinnison, H Akiyoshi, SM Frith, R Garcia, A Gettelman, JF Lamarque, T Nakamura, S Pawson, Y Yamashita, S Bekki, P Braesicke, MP Chipperfield, S Dhomse, M Marchand, E Mancini, O Morgenstern, G Pitari, D Plummer, JA Pyle, E Rozanov, J Scinocca, K Shibata, TG Shepherd, W Tian, DW Waugh - Atmospheric Chemistry and Physics (2010) 10, 9473
(DOI: 10.5194/acp-10-9473-2010)
Snow-sourced bromine and its implications for polar tropospheric ozone
X Yang, JA Pyle, RA Cox, N Theys, M Van Roozendael - Atmospheric Chemistry and Physics (2010) 10, 7763
(DOI: 10.5194/acp-10-7763-2010)


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