What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Radiative forcing in the 21st century due to ozone changes in the troposphere and the lower stratosphere - art. no. 4292
M Gauss, G Myhre, G Pitari, MJ Prather, ISA Isaksen, TK Berntsen, GP Brasseur, FJ Dentener, RG Derwent, DA Hauglustaine, LW Horowitz, DJ Jacob, M Johnson, KS Law, LJ Mickley, J Müller, P Plantevin, JA Pyle, HL Rogers, DS Stevenson, JK Sundet, M van Weele, O Wild
Journal of Geophysical Research
(2003)
108
Changes in tropospheric ozone between 2000 and 2100 modeled in a chemistry-climate model
G Zeng, JA Pyle
Geophysical Research Letters
(2003)
30
Strategies for measuring canonical tracer relationships in the stratosphere
O Morgenstern, JA Pyle
Atmospheric Chemistry and Physics
(2003)
3
Fresh air in the 21st century?
M Prather, M Gauss, T Berntsen, I Isaksen, J Sundet, I Bey, G Brasseur, F Dentener, R Derwent, D Stevenson, L Grenfell, D Hauglustaine, L Horowitz, D Jacob, L Mickley, M Lawrence, R von Kuhlmann, J Muller, G Pitari, H Rogers, M Johnson, J Pyle, K Law, M van Weele, O Wild
Geophysical Research Letters
(2003)
30
Changing ozone and changing circulation in northern mid-latitudes: Possible feedbacks?
P Braesicke, JA Pyle
Geophysical Research Letters
(2003)
30
A model study of the connection between polar and midlatitude ozone loss in the Northern Hemisphere lower stratosphere - art. no. 8323
GA Millard, AM Lee, JA Pyle
Journal of Geophysical Research
(2002)
108
Cumulative mixing inferred from stratospheric tracer relationships - art. no. 8321
O Morgenstern, AM Lee, JA Pyle
Journal of Geophysical Research
(2002)
108
The impact of meteorology on the internannual growth rate of atmospheric methane
NJ Warwick, S Bekki, KS Law, EG Nisbet, JA Pyle
Geophysical Research Letters
(2002)
29
Letter to the Editor Seasonal variations and vertical movement of the tropopause in the UTLS region
K-Y Wang, DE Shallcross, JA Pyle
Annales Geophysicae
(2002)
20
Characterising the effect of large‐scale model resolution upon calculated OH production using MOZAIC data
RA Crowther, KS Law, JA Pyle, S Bekki, HGJ Smit
Geophysical Research Letters
(2002)
29

Research Groups

Research Interest Groups

Telephone number

01223 336473