What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Ozone loss derived from balloon-borne tracer measurements in the 1999/2000 Arctic winter
AD Robinson, GA Millard, F Danis, M Guirlet, NRP Harris, AM Lee, JD McIntyre, JA Pyle, J Arvelius, S Dagnesjo, S Kirkwood, H Nilsson, DW Toohey, T Deshler, F Goutail, J-P Pommereau, JW Elkins, F Moore, E Ray, U Schmidt, A Engel, M Müller
Atmospheric Chemistry and Physics
(2005)
5
An evaluation of the performane of chemistry transport models - Part 2: Detailed comparison with two selected campaigns
D Brunner, J Staehelin, HL Rogers, MO Köhler, JA Pyle, DA Hauglustaine, L Jourdain, TK Berntsen, M Gauss, ISA Isaksen, E Meijer, P van Velthoven, G Pitari, E Mancini, V Grewe, R Sausen
Atmos. Chem. Phys.
(2005)
5
Influence of El Niño Southern Oscillation on stratosphere/ troposphere exchange and the global tropospheric ozone budget
G Zeng, JA Pyle
Geophysical Research Letters
(2005)
32
Using GOME NO2 satellite data to examine regional differences in TOMCAT model performance
NH Savage, KS Law, JA Pyle, A Richter, H Nüß, JP Burrows
Atmospheric Chemistry and Physics
(2004)
4
Refinements in the use of equivalent latitude for assimilating sporadic inhomogeneous stratospheric tracer observations, 1: Detecting transport of Pinatubo aerosol across a strong vortex edge
P Good, J Pyle
Atmospheric Chemistry and Physics
(2004)
4
Refinements in the use of equivalent latitude for assimilating sporadic inhomogeneous stratospheric tracer observations, 2: Precise altitude-resolved information about transport of Pinatubo aerosol to very high latitude
P Good, J Pyle
Atmospheric Chemistry and Physics
(2004)
4
Investigation of Arctic ozone depletion sampled over midlatitudes during the Egrett campaign of spring/summer 2000
DEM Ross, JA Pyle, NRP Harris, JD McIntyre, GA Millard, AD Robinson, R Busen
Atmospheric Chemistry and Physics
(2004)
4
Impact of a hydrogen economy on the stratosphere and troposphere studied in a 2‐D model
NJ Warwick, S Bekki, EG Nisbet, JA Pyle
Geophysical Research Letters
(2004)
31
The impact of Arctic ozone depletion on northern middle latitudes: Interannual variability and dynamical control
P Hadjinicolaou, JA Pyle
Journal of Atmospheric Chemistry
(2004)
47
An evaluation of the performance of chemistry transport models by comparison with research aircraft observations. Part 1: Concepts and overall model performance
D Brunner, J Staehelin, HL Rogers, MO Köhler, JA Pyle, D Hauglustaine, L Jourdain, TK Berntsen, M Gauss, ISA Isaksen, E Meijer, P van Velthoven, G Pitari, E Mancini, G Grewe, R Sausen
Atmos. Chem. Phys.
(2003)
3

Research Groups

Research Interest Groups

Telephone number

01223 336473