What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Athens Statement
FS Rowland, G Brasseur, RD Bojkov, M Lise, J Farman, S Godin-Beekmann, M Gonzalez, ISA Isaksen, I Karol, MJ Kurylo, M McFarland, J Pyle, R Stolarski, C Zerefos
Twenty Years of Ozone Decline Proceedings of the Symposium for the 20th Anniversary of the Montreal Protocol
(2009)
Interannual variability of tropospheric composition: The influence of changes in emissions, meteorology and clouds
A Voulgarakis, NH Savage, P Braesicke, O Wild, GD Carver, JA Pyle
Atmospheric Chemistry and Physics Discussions
(2009)
9
The sensitivity of Western European NO2 columns to interannual variability of meteorology and emissions: a model - GOME study
NH Savage, JA Pyle, P Braesicke, F Wittrock, A Richter, H Nüß, JP Burrows, MG Schultz, T Pulles, M van het Bolscher
Atmospheric Science Letters
(2008)
9
Plant spore walls as a record of long-term changes in ultraviolet-B radiation
BH Lomax, WT Fraser, MA Sephton, TV Callaghan, S Self, M Harfoot, JA Pyle, CH Wellman, DJ Beerling
Nature Geoscience
(2008)
1
Sea salt aerosol production and bromine release: Role of snow on sea ice
X Yang, JA Pyle, RA Cox
Geophysical Research Letters
(2008)
35
The World Avoided by the Montreal Protocol
O Morgenstern, P Braesicke, MM Hurwitz, FM O'Connor, AC Bushell, CE Johnson, JA Pyle
Geophysical Research Letters
(2008)
35
Radiative forcing from particle emissions by future supersonic aircraft
G Pitari, D Iachetti, E Mancini, V Montanaro, N De Luca, C Marizy, O Dessens, H Rogers, J Pyle, V Grewe, A Stenke, OA Søvde
Atmospheric Chemistry and Physics
(2008)
8
Seasonal and inter-annual variations in troposphere-to-stratosphere transport from the tropical tropopause layer
JG Levine, P Braesicke, NRP Harris, JA Pyle
Atmospheric Chemistry and Physics
(2008)
8
Impact of perturbations to nitrogen oxide emissions from global aviation
MO Köhler, G Rädel, O Dessens, KP Shine, HL Rogers, O Wild, JA Pyle
Journal of Geophysical Research
(2008)
113
Ozone trends at northern mid- and high latitudes – A European perspective
NRP Harris, E Kyrö, J Staehelin, D Brunner, S-B Andersen, S Godin-Beekmann, S Dhomse, P Hadjinicolaou, G Hansen, I Isaksen, A Jrrar, A Karpetchko, R Kivi, B Knudsen, P Krizan, J Lastovicka, J Maeder, Y Orsolini, JA Pyle, M Rex, K Vanicek, M Weber, I Wohltmann, P Zanis, C Zerefos
Annales Geophysicae
(2008)
26

Research Groups

Research Interest Groups

Telephone number

01223 336473