What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Airborne remote sensing of NO2 in the Arctic winter of 1994–1995 and comparison with a three‐dimensional chemical transport model
N Glatthor, CE Blom, T von Clarmann, H Fischer, T Gulde, C Piesch, F Erle, K Pfeilsticker, MP Chipperfield, AM Lee, JA Pyle
Journal of Geophysical Research Atmospheres
(1998)
103
Validation of an off‐line three‐dimensional chemical transport model using observed radon profiles: 2. Model results
DZ Stockwell, MA Kritz, MP Chipperfield, JA Pyle
Journal of Geophysical Research Atmospheres
(1998)
103
Effects of fluid‐dynamical stirring and mixing on the deactivation of stratospheric chlorine
DGH Tan, PH Haynes, AR MacKenzie, JA Pyle
Journal of Geophysical Research Atmospheres
(1998)
103
CFC measurements with descartes during the ILAS validation campaign - Early results
H Nilsson, K Persson, F Danis, N Harris, J Pyle
European Space Agency Special Publication ESA SP
(1997)
Effect of interannual meteorological variability on mid-latitude O-3
P Hadjinicolaou, JA Pyle, MP Chipperfield, JA Kettleborough
Geophysical Research Letters
(1997)
24
Rate constants for the reaction between OH and CH3ONO2 and C2H5ONO2 over a range of pressure and temperature
DE Shallcross, P Biggs, CE Canosa-Mas, KC Clemitshaw, MG Harrison, MRL Alañón, JA Pyle, A Vipond, RP Wayne
Journal of the Chemical Society, Faraday Transactions
(1997)
93
Temperature dependence of the ClO concentration near the stratopause
S Ghosh, JA Pyle, P Good
Journal of Geophysical Research
(1997)
102
Coupled aerosol-chemical modeling of UARS HNO3 and N2O5 measurements in the arctic upper stratosphere
S Bekki, MP Chipperfield, JA Pyle, JJ Remedios, SE Smith, RG Grainger, A Lambert, JB Kumer, JL Mergenthaler
Journal of Geophysical Research Atmospheres
(1997)
102
Implications of NOy emissions from subsonic aircraft at cruise altitude
SH Lee, M Le Dilosquer, R Singh, SE Hobbs, C Giannakopoulos, PH Plantevin, KS Law, JA Pyle, MJ Rycroft
Proceedings of the Institution of Mechanical Engineers Part G Journal of Aerospace Engineering
(1997)
211
Three-dimensional chemical forecasting: A methodology
AM Lee, GD Carver, MP Chipperfield, JA Pyle
Journal of Geophysical Research Atmospheres
(1997)
102

Research Groups

Research Interest Groups

Telephone number

01223 336473