What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

A lightweight balloon-borne gas chromatograph for in situ measurements of atmospheric halocarbons
AD Robinson, JD McIntyre, NRP Harris, JA Pyle, PG Simmonds, F Danis
Review of Scientific Instruments
(2000)
71
Large loss of total ozone during the Arctic winter of 1999/2000
B Sinnhuber, MP Chipperfield, S Davies, JP Burrows, K Eichmann, M Weber, P von der Gathen, M Guirlet, GA Cahill, AM Lee, JA Pyle
Geophysical Research Letters
(2000)
27
A three‐dimensional model calculation of the ozone depletion potential of 1‐bromopropane (1‐C3H7Br)
CH Bridgeman, JA Pyle, DE Shallcross
Journal of Geophysical Research Atmospheres
(2000)
105
Modeled Arctic ozone depletion in winter 1997/1998 and comparison with previous winters
M Guirlet, MP Chipperfield, JA Pyle, F Goutail, JP Pommereau, E Kyrö
Journal of Geophysical Research: Atmospheres
(2000)
105
A three‐dimensional modeling study of the correlations of 210Pb with HNO3 and peroxyacetylnitrate (PAN) at remote oceanic sites
C Giannakopoulos, MP Chipperfield, KS Law, P Plantevin, JA Pyle, DE Shallcross
Journal of Geophysical Research Atmospheres
(2000)
105
Evaluation of a Lagrangian box model using field measurements from EASE (Eastern Atlantic Summer Experiment) 1996
MJ Evans, DE Shallcross, KS Law, JOF Wild, PG Simmonds, TG Spain, P Berrisford, J Methven, AC Lewis, JB McQuaid, MJ Pilling, BJ Bandy, SA Penkett, JA Pyle
Atmospheric Environment
(2000)
34
DESCARTES: A novel lightweight balloon-borne instrument for measurement of halocarbons
F Danis, NRP Harris, WH Taylor, JD McIntyre, PG Simmonds, JA Pyle
Review of Scientific Instruments
(2000)
71
Validation and intercomparison of wet and dry deposition schemes using Pb-210 in a global three-dimensional off-line chemical transport model
C Giannakopoulos, MP Chipperfield, KS Law, JA Pyle
Journal of Geophysical Research
(1999)
104
Implementation of a convective atmospheric boundary layer scheme in a tropospheric chemistry transport model
K Wang, JA Pyle, MG Sanderson, C Bridgeman
Journal of Geophysical Research
(1999)
104
Intercomparison of measured and modelled BrO slant column amounts for the Arctic winter and spring 1994/95
U Frieß, MP Chipperfield, H Harder, C Otten, U Platt, J Pyle, T Wagner, K Pfeilsticker
Geophysical Research Letters
(1999)
26

Research Groups

Research Interest Groups

Telephone number

01223 336473