What I do

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling

The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling

We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions

These interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements

We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

SENSITIVITY OF SUPERSONIC AIRCRAFT MODELING STUDIES TO HNO3 PHOTOLYSIS RATE
AE Jones, S Bekki, JA Pyle
Geophysical Research Letters
(2012)
20
Potential impact of combined NOx and SOx emissions from future high speed civil transport aircraft on stratospheric aerosols and ozone
S Bekki, JA Pyle
Geophysical Research Letters
(2012)
20
The bliss measurements of NO2: Some new insights
DJ Lary, JA Pyle, CR Webster, RD May
Geophysical Research Letters
(2012)
18
THEORETICAL INTERPRETATION OF N2O5 MEASUREMENTS
R Toumi, JA Pyle, CR Webster, RD May
Geophysical Research Letters
(2012)
18
Modelling future changes to the stratospheric source gas injection of biogenic bromocarbons
R Hossaini, MP Chipperfield, S Dhomse, C Ordóñez, A Saiz‐Lopez, NL Abraham, A Archibald, P Braesicke, P Telford, N Warwick, X Yang, J Pyle
Geophysical Research Letters
(2012)
39
Tropical convective transport and the Walker circulation
JS Hosking, MR Russo, P Braesicke, JA Pyle
Atmospheric Chemistry and Physics
(2012)
12
2-DIMENSIONAL MODELING OF THE NORTHERN-HEMISPHERE HIGH-LATITUDE LOWER STRATOSPHERE
MP Chipperfield, JA Pyle
Journal of Geophysical Research: Atmospheres
(2012)
95
On the atmospheric impact of launching the Ariane 5 rocket
AE Jones, S Bekki, JA Pyle
Journal of Geophysical Research
(2012)
100
Observations of CH4 and N2O by the Nimbus 7 SAMS: a comparison with in situ data and two-dimensional numerical model calculations.
RL Jones, JA Pyle
Journal of Geophysical Research: Atmospheres
(2012)
89
Active nitrogen partitioning and the nighttime formation of N2O5 in the stratosphere: Simultaneous in situ measurements of NO, NO2, HNO3, O3, and N2O using the BLISS diode laser spectrometer
CR Webster, RD May, R Toumi, JA Pyle
Journal of Geophysical Research: Atmospheres
(2012)
95

Research Groups

Research Interest Groups

Telephone number

01223 336473