Department of Chemistry

portrait of Professor John Pyle FRS

Professor John Pyle FRS

St Catharine's College

Groups: Atmospheric group website

Telephone: 01223 336473

E-mail: john.pyle@atm.ch.cam.ac.uk

My research involves the use of state-of-the-art numerical models, run on supercomputers, to study the processes controlling the present state of the atmosphere and its evolution. A NERC Unit, the Atmospheric Chemistry Modelling Support Unit, is incorporated into the group.

Current research activities include:

Stratospheric Modelling. The chemistry, dynamics and radiative transfer of the stratosphere are being studied using a number of numerical models. Three particular problems being tackled are (i) the rapid depletion of ozone found recently in the polar spring, the so-called 'ozone hole', (ii) the more gradual decline in northern hemisphere ozone levels (which we have recently ascribed partly to long-term changes in atmospheric flow, and (iii) the effect on stratospheric ozone of increasing concentrations of CO2, CH4, N2O and the chlorofluorocarbons.

Tropospheric Modelling. We have developed a range of models for studying the chemistry of the lower atmosphere, from complex 3D models to models based on air parcel trajectories. A major research theme is the changing oxidizing capacity of the troposphere (the ability of the troposphere to cleanse itself of pollution). An important part of our work includes involvement in field campaigns.

Chemistry/climate interactions have become a major research topic in recent years. We have included a detailed chemistry package into the Met Office's climate model, to study composition change since the industrial revolution and into the future. We have calculated the change in surface ozone at the end of this century, under certain assumptions about changing industrial emissions. The change is very climate-dependent, but shows massive increases (which are expected to lead to major health problems) over some of the continents.

Atmospheric composition measurements. We have developed lightweight gas chromatography instruments to measure halocarbons. These have been deployed from balloons and high-flying research aircraft.

Many of the problems addressed are of an interdisciplinary nature. Members of the group, which numbers about 20 postdoctoral researchers and students, come from a wide range of backgrounds in mathematics and physical science. Within Cambridge we collaborate closely with scientists at the Department of Applied Mathematics and Theoretical Physics.

Publications

Ozone loss in middle latitudes and the role of the Arctic polar vortex
JA PYLE - Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences (1995) 352, 241
(DOI: 10.1098/rsta.1995.0067)
THE VARIABILITY OF CLONO2 AND HNO3 IN THE ARCTIC POLAR VORTEX - COMPARISON OF TRANSALL MICHELSON INTERFEROMETER FOR PASSIVE ATMOSPHERIC SOUNDING MEASUREMENTS AND 3-DIMENSIONAL MODEL RESULTS
MP CHIPPERFIELD, JA PYLE, CE BLOM, N GLATTHOR, M HOPFNER, T GULDE, C PIESCH, P SIMON - Journal of Geophysical Research (1995) 100, 9115
(DOI: 10.1029/94JD02309)
Modelling the global sources and sinks of radiatively active gases
JA PYLE, P BROWN, S BEKKI, GD CARVER, KS LAW, DZ STOCKWELL - Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences (1995) 351, 397
(DOI: 10.1098/rsta.1995.0042)
ESTIMATION OF HETEROGENEOUS REACTION-RATES FOR STRATOSPHERIC TRACE GASES WITH PARTICULAR REFERENCE TO THE DIFFUSIONAL UPTAKE OF HCL AND CLONO2 BY POLAR STRATOSPHERIC CLOUDS
S GHOSH, D LARY, JA PYLE - Annales Geophysicae (1995) 13, 406
(DOI: 10.1007/s005850050175)
STRATOSPHERIC OCLO MEASUREMENTS AS A POOR QUANTITATIVE INDICATOR OF CHLORINE ACTIVATION
J SESSLER, MP CHIPPERFIELD, JA PYLE, R TOUMI - Geophysical Research Letters (1995) 22, 687
(DOI: 10.1029/95GL00202)
Lessons for the future from coordinated European stratospheric campaigns
JA Pyle, NRP Harris - Physics and Chemistry of the Earth (1995) 20, 5
(DOI: 10.1016/0079-1946(95)00003-S)
Early modelling results from the SESAME and ASHOE campaigns
JA Pyle, MP Chipperfield, I KilbaneDawe, AM Lee, RM Stimpfle, D Kohn, W Renger, JW Waters - Faraday Discussions (1995) 100, 371
(DOI: 10.1039/fd9950000371)
3-DIMENSIONAL TRACER INITIALIZATION AND GENERAL DIAGNOSTICS USING EQUIVALENT PV LATITUDE-POTENTIAL-TEMPERATURE COORDINATES
DJ LARY, MP CHIPPERFIELD, JA PYLE, WA NORTON, LP RIISHOJGAARD - Quarterly Journal - Royal Meteorological Society (1995) 121, 187
(DOI: 10.1002/qj.49712152109)
EFFECT OF OZONE DEPLETION ON ATMOSPHERIC CH4 AND CO CONCENTRATIONS
S BEKKI, KS LAW, JA PYLE - Nature (1994) 371, 595
(DOI: 10.1038/371595a0)
A 2-DIMENSIONAL MODELING STUDY OF THE VOLCANIC-ERUPTION OF MOUNT-PINATUBO
S BEKKI, JA PYLE - Journal of Geophysical Research (1994) 99, 18861
(DOI: 10.1029/94JD00667)


General


Research Interests


Teaching


Personal


Publications

Funding


Funding 

Further Funding Information