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Steffen Emge

Research Associate

Contact information

mail se359 "at" cam.ac.uk

       about.me/se359

ORCID iD iconorcid.org/0000-0001-8613-9465

 

Current Research topics

  • Coatings
  • Solid electrolytes
  • All-solid-state batteries
  • (PFG-)NMR

 

Previous research interests

  • Organic electrosynthesis
  • Supercapacitors
  • Ionic liquids
  • eQCM

 

Publications

[1]  Electrochemical selenium- and iodonium-initiated cyclisation of hydroxy-functionalised 1,4-dienes

P. Röse, S. Emge, J. Yoshida, G. Hilt, Beilstein J. Org. Chem. 2015, 11, 174

DOI: 10.3762/bjoc.11.18

[2] Structural and Mechanistic Insights into Fast Lithium-Ion Conduction in Li4SiO4–Li3PO4 Solid Electrolytes

Y. Deng, C. Eames, J.N. Chotard, F. Lalère, V. Seznec, S. Emge, O. Pecher, C.P. Grey, C. Masquelier, M.S. Islam, JACS 2015, 137, 9136

DOI: 10.1021/jacs.5b04444

[3] Efficient Oxidative Coupling of Arenes via Electrochemical Regeneration of 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) under Mild Reaction Conditions

P. Röse, S. Emge, C.A. König, G. Hilt, Adv. Synth. Catal. 2017, 359,1359

DOI: 10.1002/adsc.201601331

[4] Quantitative Information about Electrosorption of Ionic Liquids in Carbon Nanopores from Electrochemical Dilatometry and Quartz Crystal Microbalance Measurements

N. Jäckel, S. P. Emge, B. Krüner, B. Roling, V. Presser, J. Phys. Chem. C 2017, 121, 19120

DOI: 10.1021/acs.jpcc.7b06915

[5] Elucidating Lithium-Ion and Proton Dynamics in Anti-Perovskite Solid Electrolytes

J. A. Dawson, T. Attari, H. Chen, S. Emge, K. E Johnston, Saiful Islam, Energy Environ. Sci. 2018, 11, 2993

DOI: 10.1039/C8EE00779A

[6] 7Li NMR Chemical Shift Imaging to Detect Microstructural Growth of Lithium in All Solid-State Batteries

L. E. Marbella, S. Zekoll, J. Kasemchainan, S. P. Emge, P. G. Bruce, C. P. Grey, Chem. Mater. 2019,  31, 2762

DOI: 10.1021/acs.chemmater.8b04875

[7] Al/Ga-Doped Li7La3Zr2O12 Garnets as Li-Ion Solid-State Battery Electrolytes: Atomistic Insights into Local Coordination Environments and Their Influence on 17O, 27Al, and 71Ga NMR Spectra

S. P. Emge, B. Karasulu, M. F. Groh, C. P. Grey, A. J. Morris J. Am. Chem. Soc. 2020, 142, 3132

DOI: 10.1021/jacs.9b12685

[8] Establishing Ultra-Low Activation Energies for Lithium Transport in Garnet Electrolytes

F. M. Pesci , A. Bertei, R. H Brugge, S. P. Emge, A.K. O. Hekselman, L. E Marbella, C. P. Grey, A. Aguadero ACS Appl. Mater. Interfaces 2020, 12, 32806 

DOI: 10.1021/acsami.0c08605

[9] Bulk Fatigue Induced by Surface Reconstruction in Layered Ni-Rich Oxide Cathodes for Li-ion Batteries

C. Xu, K. Märker, J. Lee, A Mahadevegowda, PJ Reeves, S. J. Day, M. F. Groh, S. P. Emge, C. Ducati, B. Layla Mehdi, C. C. Tang, C. P. Grey – Nature Materials 2021 20, 84

DOI: 10.1038/s41563-020-0767-8

[10] Under Pressure: Mechanochemical Effects on Structure and Ion Conduction in the Sodium-Ion Solid Electrolyte Na3PS4

T Famprikis, ÖU Kudu, JA Dawson, P Canepa, F Fauth, E Suard, M Zbiri, D Dambournet, OJ Borkiewicz, H Bouyanfif, SP Emge, S Cretu, J-N Chotard, CP Grey, WG Zeier, MS Islam, C Masquelier – J Am Chem Soc 2020 142, 18422

DOI: 10.1021/jacs.0c06668

[11] Impact of orientational glass formation and local strain on photo-induced halide segregation in hybrid metal-halide perovskites

TWJ van de Goor, Y Liu, S Feldmann, SA Bourelle, T Neumann, T Winkler, ND Kelly, C Liu, MA Jones, SP Emge, RH Friend, B Monserrat, F Deschler, SE Dutton – The Journal of Physical Chemistry C 2021 125, 15025

DOI:10.1021/acs.jpcc.1c03169

 

Preprints

A directed sampling approach for modelling the structural and electronic properties of amorphous alumina

A. F. Harper, S. P. Emge ,P. C. M. M. Magusin, C. P. Grey, A. J. Morris, 2021 DOI: 10.33774/chemrxiv-2021-qjzbj

 

Publications

Impact of Orientational Glass Formation and Local Strain on Photo-Induced Halide Segregation in Hybrid Metal-Halide Perovskites
TWJ van de Goor, Y Liu, S Feldmann, SA Bourelle, T Neumann, T Winkler, ND Kelly, C Liu, MA Jones, SP Emge, RH Friend, B Monserrat, F Deschler, SE Dutton
– The Journal of Physical Chemistry C: Energy Conversion and Storage, Optical and Electronic Devices, Interfaces, Nanomaterials, and Hard Matter
(2021)
125,
15025
(doi: 10.1021/acs.jpcc.1c03169)
SOLID-STATE NMR INVESTIGATION OF STRUCTURE AND DYNAMICS OF SOLID ELECTROLYTES AND COATINGS FOR LI-ION BATTERY APPLICATIONS
S Emge
(2020)
(doi: 10.17863/CAM.65611)
Under Pressure: Mechanochemical Effects on Structure and Ion Conduction in the Sodium-Ion Solid Electrolyte Na3PS4.
T Famprikis, ÖU Kudu, JA Dawson, P Canepa, F Fauth, E Suard, M Zbiri, D Dambournet, OJ Borkiewicz, H Bouyanfif, SP Emge, S Cretu, J-N Chotard, CP Grey, WG Zeier, MS Islam, C Masquelier
– Journal of the American Chemical Society
(2020)
142,
18422
(doi: 10.1021/jacs.0c06668)
Bulk fatigue induced by surface reconstruction in layered Ni-rich cathodes for Li-ion batteries.
C Xu, K Märker, J Lee, A Mahadevegowda, PJ Reeves, SJ Day, MF Groh, SP Emge, C Ducati, B Layla Mehdi, CC Tang, CP Grey
– Nature materials
(2020)
20,
84
(doi: 10.1038/s41563-020-0767-8)
Establishing Ultralow Activation Energies for Lithium Transport in Garnet Electrolytes
FM Pesci, A Bertei, RH Brugge, SP Emge, AKO Hekselman, LE Marbella, CP Grey, A Aguadero
– ACS Appl Mater Interfaces
(2020)
12,
32806
(doi: 10.1021/acsami.0c08605)
Al/Ga-Doped Li7La3Zr2O12 Garnets as Li-Ion Solid-State Battery Electrolytes: Atomistic Insights into Local Coordination Environments and Their Influence on 17O, 27Al, and 71Ga NMR Spectra
B Karasulu, SP Emge, MF Groh, CP Grey, AJ Morris
– J Am Chem Soc
(2020)
142,
3132
(doi: 10.1021/jacs.9b12685)
7Li NMR Chemical Shift Imaging To Detect Microstructural Growth of Lithium in All-Solid-State Batteries
LE Marbella, S Zekoll, J Kasemchainan, SP Emge, PG Bruce, CP Grey
– Chemistry of materials : a publication of the American Chemical Society
(2019)
31,
2762
(doi: 10.1021/acs.chemmater.8b04875)
Elucidating lithium-ion and proton dynamics in anti-perovskite solid electrolytes
JA Dawson, TS Attari, H Chen, SP Emge, KE Johnston, MS Islam
– Energy and Environmental Science
(2018)
11,
2993
(doi: 10.1039/c8ee00779a)
Quantitative Information about Electrosorption of Ionic Liquids in Carbon Nanopores from Electrochemical Dilatometry and Quartz Crystal Microbalance Measurements
N Jaeckel, SP Emge, B Kruener, B Roling, V Presser
– Journal of Physical Chemistry C
(2017)
121,
19120
(doi: 10.1021/acs.jpcc.7b06915)
Efficient Oxidative Coupling of Arenes via Electrochemical Regeneration of 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) under Mild Reaction Conditions
P Röse, S Emge, CA König, G Hilt
– Advanced Synthesis and Catalysis
(2017)
359,
1359
(doi: 10.1002/adsc.201601331)
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