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Yusuf Hamied Department of Chemistry

 

Research Summary

Current position. Marie Curie Fellow at Reisner Lab working in the development of hybrid materials-enzymes for solar fuel production.

Brief career summary. I began my research career at the University of Girona, where my Master thesis (thanks to a Collaboration Fellowship from the Spanish Ministry) focused on the study of water oxidation with well-defined tetra- and pentacoordinate ruthenium complexes having aminopyridyl ligand scaffolds. The work combined experimental reactivity and mechanistic studies with computational modelling and was carried out under the joint supervision of Prof. Miquel Costas and Prof. Julio Lloret. In November 2014 I joined ICIQ as a FPU doctoral student together with my advisor Prof. Julio Lloret, with whom we set up a new research laboratory from scratch. My doctoral work sought a fundamental understanding of the mechanisms involved in artificial photosynthetic schemes and their application to store sunlight energy into chemical bonds, as well as to develop new greener and sustainable methodologies to produce solar fuels and fine chemicals.

In September 2019, I started as a BBSRC (Biotechnology and Biological Sciences Research Council) postdoctoral researcher at the group of Prof. Reisner at the University of Cambridge. My research focussed in the development of material-protein hybrids for solar fuel synthesis. 

In March 2020, I was awarded a Marie Curie IF fellowship (MSCA-IF-2019 ref: 890745-SmArtC), so I have just been appointed Marie Curie Fellow in the same group and now my research focusses in developing compartmentalised systems for semiartificial CO2 reduction. 

Publications

  • Roadmap towards solar fuel synthesis at the water interface of liposome membranes

A Pannwitz, DM Klein, S Rodríguez-Jiménez, C Casadevall, H Song, E Reisner, L Hammarström, S Bonnet 

Chem Soc Rev (2021); DOI: 10.1039/d0cs00737d


  • Visible‐Light Promoted C–O Bond Formation with an Integrated Carbon Nitride–Nickel Heterogeneous Photocatalyst

A, Vijeta, C. Casadevall, S. Roy and E. Reisner 

ACIE (2021) doi.org/10.1002/anie.202016511


  • Electrocatalytic water oxidation with α-[Fe(mcp)(OTf)2] and analogues

S. d’Agostini, K. Kottrup, C.Casadevall, I. Gamba, M. Costas, J. Lloret-Fillol, D. Hatterscheid 

ACS Catalysts, online doi.org/10.1021/acscatal.0c05439.


  • The synergy between the CsPbBr3 nanoparticle surface and the organic ligand becomes manifest in a demanding carbon–carbon coupling reaction

I.Rosa-Pardo, C.Casadevall, L.Schmidt, M.Claros, R. E. Galian, J. Lloret-Fillol, J. Pérez-Prieto

Chem. Commun. 2020, 56, 5026. doi.org/10.1039/D0CC01339K


  • A Unified Electro- and Photocatalytic CO2 to CO Reduction Mechanism with Aminopyridine Cobalt Complexes

S.Fernández, F.Franco, C.Casadevall, V.Martin-Diaconescu, J. M. Luis, J. Lloret-.Fillol;

J. Am. Chem. Soc. 2020, 142 (1), 120. doi.org/10.1021/jacs.9b06633


  • Current opinion in artificial photosynthesis with molecular catalysts 

C. Casadevall*

EAES, ISSN: 2578-0336, 2020.


  • Water Oxidation Catalysis with Well-defined Molecular Iron Complexes

C.Casadevall, A.Bucci, M.Costas, J.Lloret-Fillol;

 Adv. Inorg. Chem. 74, 2019, 151. doi.org/10.1016/bs.adioch.2019.03.004


  • Improved Electro- and Photocatalytic Water Reduction by Confined Cobalt Catalysts in Streptavidin

A.Call±, C.Casadevall±, A.Romero-Rivera, D.J.Sommer, S. Osuna, G. Ghirlanda, and J. Lloret-Fillol,

ACS Catal. 2019, 9 (7), 5837. ± equal contribution doi.org/10.1021/acscatal.8b04981


  • Design of Iron Coordination Complexes as Highly Active Homogenous Water Oxidation Catalysts by Deuteration of Oxidation-Sensitive Sites

Z.Codolà, I.Gamba, F.Acuña-Parés, C.Casadevall, M. Clémancey, J-M. Latour, J. M. Luis, M. Costas, J. Lloret-Fillol;

J. Am. Chem. Soc, 2019, 141 (1), 323.  doi.org/10.1021/jacs.8b10211


  • Dual cobalt-copper light-driven catalytic reduction of aldehydes and aromatic ketones in aqueous media

A.Call±, C.Casadevall±, F.Acuña-Parés, A.Casitas, J.Lloret-Fillol;

Chem. Sci. 2017, 8 (7), 4739. ± equal contribution doi.org/10.1039/C7SC01276D

Front cover, Highlighted in Chemistry World and Chemistry Views and This article is part of the themed collection: Most downloaded articles of 2017: Energy and Catalysis


  • Catalizadores para la conversión de la energía solar en enlaces químicos

C. Casadevall, A. Call, Z. Codolà, F. Acuña-Parés, J. Lloret-Fillol;

An. Quim. 2016, 112 (3), 133. 


  • Spectroscopic, Electrochemical and Computational Characterisation of Ru Species Involved in Catalytic Water Oxidation: Evidence for a [RuV(O)(Py2Metacn)] Intermediate

C.Casadevall, Z.Codola, M.Costas, J.Lloret-Fillol,

Chem. Eur. J. 2016, 22 (29), 10111. doi.org/10.1002/chem.201600584

Research Group

Telephone number

01223 336396 (shared)

Email address

cc2036@cam.ac.uk